Poly L-Dopa/poly(ethylenedioxythiophene) as a novel mussel-inspired electroactive binder for environmentally friendly hybrid supercapacitors
3,4-Dihydroxy-L-phenylalanine and ethylenedioxythiophene
were chemically copolymerized via an oxidative process in aqueous solution.
The copolymer was used as a novel mussel-inspired electroactive binder in
conjunction with a nickel-based metal organic frame work for fabrication of
environmentally friendly supercapacitors. The binder, in addition to the
sticking effect, contributes to electric charge storing via the redox
process of catechol moieties of poly(3,4-dihydroxy-L-phenylalanine) and also
the formation of a high charge-storing double layer due to the presence of
poly(ethylenedioxythiophene). Cyclic voltammetry, charge/discharge
measurements, and electrochemical impedance spectrometry showed that the
hybrid supercapacitors based on Ni-benzidine MOF with the new electroactive
binder exhibit very high specific capacitance (770 F g−1−1^{-1} at 1 A/g) and
remarkable capacitance retention of more than 94% after 1000 cycles and
86% after 5000 cycles at high current density of 5 A g−1−1^{-1}.
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